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Self-assembled flower-like ZnIn2S4 coupled with g-C3N4@ ZIF-67 heterojunction for improved photocatalytic hydrogen performance

Self-assembled flower-like ZnIn2S4 coupled with g-C3N4@ ZIF-67 heterojunction for improved photocatalytic hydrogen performance

저자

Ramanadha Mangiri, K Subramanyam, Junbeum Lee, Min Kyeong Lee, Chaehyeon Lee, Mohd Shahnawaz Khan, Nipa Roy, Sang Woo Joo, Eunhyea Chung

저널 정보

Surfaces and Interfaces

출간연도

2024/6/1

Enhancing the photocatalytic performance of ZnIn2S4 (ZIS) photocatalysts is a formidable task due to their structural and compositional challenges. In this investigation, a flower-like ZnIn2S4 was synthesized, coupled with a g-C3N4@ZIF-67 heterojunction, using a hydrothermal approach. Incorporating carbon-based composites led to a special electron trapping effect, effectively mitigating the photocatalytic limitations arising from the broader band gap, weak conductivity, and poor photocatalytic response activity of GCN. Consequently, introducing carbon-based composites facilitated the construction of a stable photocatalytic heterojunction. The formed heterojunction was characterized using XRD, FE-SEM, FE-TEM, EDS, XPS, electrochemical and Mott-Schottky measurements. The composite heterojunction photocatalyst, showcasing a bifunctional design, exhibited outstanding hydrogen production performance …